Local structure and electrochemistry of LiNiyMnyCo1−2yO2 electrode materials for Li-ion batteries
Identifieur interne : 000723 ( Main/Exploration ); précédent : 000722; suivant : 000724Local structure and electrochemistry of LiNiyMnyCo1−2yO2 electrode materials for Li-ion batteries
Auteurs : K. Ben Kamel [Tunisie] ; N. Amdouni [Tunisie] ; A. Abdel-Ghany [France] ; K. Zaghib [Canada] ; A. Mauger [France] ; F. Gendron [France] ; C. M. Julien [France]Source :
- Ionics [ 0947-7047 ] ; 2008.
English descriptors
Abstract
A series of LiNixMnyCozO2 (x=y, z=1−2y) oxides have been synthesized by “chimie douce” and investigated as positive electrodes in rechargeable lithium batteries. Layered LiNiyMnyCo1−2yO2 materials with high homogeneity and crystallinity were synthesized using the wet-chemical method assisted by carboxylic acid as the polymeric agent. The long range and local structural properties are investigated with experiments including Xray diffraction, Fourier transform infrared spectroscopy, and electron paramagnetic resonance spectroscopy. The evolution of the structure is discussed as a function of the cobalt content that confers layer-like behavior on the framework. Electrochemical performance of LiNiyMnyCo1−2yO2 oxides is tested in cells using nonaqueous 1 M LiPF6 dissolved in ethylene carbonate–diethyl carbonate. Charge–discharge profiles are investigated as a function of the rate capability and the voltage window. A relation is found between the gravimetric capacity and the cation disorder of the positive electrode as indicated by structural analysis. Fast lithium extraction attributed to the larger interslab space has been observed in the cobalt-rich oxides
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DOI: 10.1007/s11581-007-0167-y
Affiliations:
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Zaghib</name><affiliation wicri:level="1"><hal:affiliation type="institution" xml:id="struct-301422" status="VALID"><orgName>Institut de Recherche d'Hydro-Québec [Varennes]</orgName><orgName type="acronym">IREQ</orgName><desc><address><addrLine>1800 Boulevard Lionel Boulet, Varennes, QC J3X 1S1</addrLine><country key="CA"></country></address><ref type="url">http://www.hydroquebec.com/innovation/fr/institut-recherche.html</ref></desc></hal:affiliation><country>Canada</country></affiliation></author><author><name sortKey="Mauger, A" sort="Mauger, A" uniqKey="Mauger A" first="A." last="Mauger">A. Mauger</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-3204" status="OLD"><orgName>Institut de minéralogie et de physique des milieux condensés</orgName><orgName type="acronym">IMPMC</orgName><desc><address><addrLine>Campus Boucicaut 140, rue de Lourmel 75015 - Paris</addrLine><country key="FR"></country></address><ref type="url">http://www.impmc.jussieu.fr/</ref></desc><listRelation><relation active="#struct-93591" type="direct"></relation><relation active="#struct-300063" type="direct"></relation><relation active="#struct-300301" type="direct"></relation><relation name="UMR7590" active="#struct-441569" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-93591" type="direct"><org type="institution" xml:id="struct-93591" status="VALID"><orgName>Université Pierre et Marie Curie - Paris 6</orgName><orgName type="acronym">UPMC</orgName><desc><address><addrLine>4 place Jussieu - 75005 Paris</addrLine><country key="FR"></country></address><ref type="url">http://www.upmc.fr/</ref></desc></org></tutelle><tutelle active="#struct-300063" type="direct"><org type="institution" xml:id="struct-300063" status="VALID"><orgName>IPG PARIS</orgName><desc><address><country key="FR"></country></address></desc></org></tutelle><tutelle active="#struct-300301" type="direct"><org type="institution" xml:id="struct-300301" status="VALID"><orgName>Université Paris Diderot - Paris 7</orgName><orgName type="acronym">UP7</orgName><desc><address><addrLine>5 rue Thomas-Mann - 75205 Paris cedex 13</addrLine><country key="FR"></country></address><ref type="url">http://www.univ-paris-diderot.fr</ref></desc></org></tutelle><tutelle name="UMR7590" active="#struct-441569" type="direct"><org type="institution" xml:id="struct-441569" status="VALID"> <idno type="ISNI">0000000122597504</idno> <idno type="IdRef">02636817X</idno> <orgName>Centre National de la Recherche Scientifique</orgName> <orgName type="acronym">CNRS</orgName> <date type="start">1939-10-19</date> <desc> <address> <country key="FR"></country> </address> <ref type="url">http://www.cnrs.fr/</ref> </desc></org></tutelle></tutelles></hal:affiliation><country>France</country></affiliation></author><author><name sortKey="Gendron, F" sort="Gendron, F" uniqKey="Gendron F" first="F." last="Gendron">F. Gendron</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-101592" status="VALID"><idno type="RNSR">199712634A</idno><orgName>Institut des Nanosciences de Paris</orgName><orgName type="acronym">INSP</orgName><desc><address><addrLine>Université Pierre et Marie Curie Case 840 4 place Jussieu 75252 Paris Cedex 05</addrLine><country key="FR"></country></address><ref type="url">http://www.insp.upmc.fr</ref></desc><listRelation><relation active="#struct-93591" type="direct"></relation><relation name="UMR7588" active="#struct-441569" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-93591" type="direct"><org type="institution" xml:id="struct-93591" status="VALID"><orgName>Université Pierre et Marie Curie - Paris 6</orgName><orgName type="acronym">UPMC</orgName><desc><address><addrLine>4 place Jussieu - 75005 Paris</addrLine><country key="FR"></country></address><ref type="url">http://www.upmc.fr/</ref></desc></org></tutelle><tutelle name="UMR7588" active="#struct-441569" type="direct"><org type="institution" xml:id="struct-441569" status="VALID"> <idno type="ISNI">0000000122597504</idno> <idno type="IdRef">02636817X</idno> <orgName>Centre National de la Recherche Scientifique</orgName> <orgName type="acronym">CNRS</orgName> <date type="start">1939-10-19</date> <desc> <address> <country key="FR"></country> </address> <ref type="url">http://www.cnrs.fr/</ref> </desc></org></tutelle></tutelles></hal:affiliation><country>France</country></affiliation></author><author><name sortKey="Julien, C M" sort="Julien, C M" uniqKey="Julien C" first="C. M." last="Julien">C. M. Julien</name><affiliation wicri:level="1"><hal:affiliation type="laboratory" xml:id="struct-101592" status="VALID"><idno type="RNSR">199712634A</idno><orgName>Institut des Nanosciences de Paris</orgName><orgName type="acronym">INSP</orgName><desc><address><addrLine>Université Pierre et Marie Curie Case 840 4 place Jussieu 75252 Paris Cedex 05</addrLine><country key="FR"></country></address><ref type="url">http://www.insp.upmc.fr</ref></desc><listRelation><relation active="#struct-93591" type="direct"></relation><relation name="UMR7588" active="#struct-441569" type="direct"></relation></listRelation><tutelles><tutelle active="#struct-93591" type="direct"><org type="institution" xml:id="struct-93591" status="VALID"><orgName>Université Pierre et Marie Curie - Paris 6</orgName><orgName type="acronym">UPMC</orgName><desc><address><addrLine>4 place Jussieu - 75005 Paris</addrLine><country key="FR"></country></address><ref type="url">http://www.upmc.fr/</ref></desc></org></tutelle><tutelle name="UMR7588" active="#struct-441569" type="direct"><org type="institution" xml:id="struct-441569" status="VALID"> <idno type="ISNI">0000000122597504</idno> <idno type="IdRef">02636817X</idno> <orgName>Centre National de la Recherche Scientifique</orgName> <orgName type="acronym">CNRS</orgName> <date type="start">1939-10-19</date> <desc> <address> <country key="FR"></country> </address> <ref type="url">http://www.cnrs.fr/</ref> </desc></org></tutelle></tutelles></hal:affiliation><country>France</country></affiliation></author></analytic><idno type="DOI">10.1007/s11581-007-0167-y</idno><series><title level="j">Ionics</title><idno type="ISSN">0947-7047</idno><imprint><date type="datePub">2008</date></imprint></series></biblStruct></sourceDesc></fileDesc><profileDesc><textClass><keywords scheme="mix" xml:lang="en"><term>Intercalation compounds</term><term>Layered structure</term><term>Li-ion batteries</term><term>Transition-metal oxides</term></keywords></textClass></profileDesc></teiHeader><front><div type="abstract" xml:lang="en">A series of LiNixMnyCozO2 (x=y, z=1−2y) oxides have been synthesized by “chimie douce” and investigated as positive electrodes in rechargeable lithium batteries. Layered LiNiyMnyCo1−2yO2 materials with high homogeneity and crystallinity were synthesized using the wet-chemical method assisted by carboxylic acid as the polymeric agent. The long range and local structural properties are investigated with experiments including Xray diffraction, Fourier transform infrared spectroscopy, and electron paramagnetic resonance spectroscopy. The evolution of the structure is discussed as a function of the cobalt content that confers layer-like behavior on the framework. Electrochemical performance of LiNiyMnyCo1−2yO2 oxides is tested in cells using nonaqueous 1 M LiPF6 dissolved in ethylene carbonate–diethyl carbonate. Charge–discharge profiles are investigated as a function of the rate capability and the voltage window. A relation is found between the gravimetric capacity and the cation disorder of the positive electrode as indicated by structural analysis. Fast lithium extraction attributed to the larger interslab space has been observed in the cobalt-rich oxides</div></front></TEI><affiliations><list><country><li>Canada</li><li>France</li><li>Tunisie</li></country></list><tree><country name="Tunisie"><noRegion><name sortKey="Ben Kamel, K" sort="Ben Kamel, K" uniqKey="Ben Kamel K" first="K." last="Ben Kamel">K. Ben Kamel</name></noRegion><name sortKey="Amdouni, N" sort="Amdouni, N" uniqKey="Amdouni N" first="N." last="Amdouni">N. Amdouni</name></country><country name="France"><noRegion><name sortKey="Abdel Ghany, A" sort="Abdel Ghany, A" uniqKey="Abdel Ghany A" first="A." last="Abdel-Ghany">A. Abdel-Ghany</name></noRegion><name sortKey="Gendron, F" sort="Gendron, F" uniqKey="Gendron F" first="F." last="Gendron">F. Gendron</name><name sortKey="Julien, C M" sort="Julien, C M" uniqKey="Julien C" first="C. M." last="Julien">C. M. Julien</name><name sortKey="Mauger, A" sort="Mauger, A" uniqKey="Mauger A" first="A." last="Mauger">A. Mauger</name></country><country name="Canada"><noRegion><name sortKey="Zaghib, K" sort="Zaghib, K" uniqKey="Zaghib K" first="K." last="Zaghib">K. Zaghib</name></noRegion></country></tree></affiliations></record>Pour manipuler ce document sous Unix (Dilib)
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